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Chem. Phys. 90, 3214 (1989). 25. M. Rittby and R. J. Bartlett, unpublished data. 26. W. P. Kraemer, P. R. Bunker and M. Yoshimine, J. Mol. Spectrosc. 107, 1 9 1 ( 1984). 27. F. J. Kohl and C. A. Steams, J. Chem. Phys. 52 , 63 1 ( 1970). 28. K. K. Sunil, A. Orendt and K. D. Jordan, Chem. Phys. 89, 245 (1984). 29. H. Sasada, T. Amano, C. Jarman and P. F. Bernath, J. Chem. Phys. 94, 240 1 (199 1). J. Reynolds (Editor) © 1 993 Elsevier Science Publishers B. V. All rights reserved. N. M. Neumark* 3.

R. Bunker and M. Yoshimine, J. Mol. Spectrosc. 107, 1 9 1 ( 1984). 27. F. J. Kohl and C. A. Steams, J. Chem. Phys. 52 , 63 1 ( 1970). 28. K. K. Sunil, A. Orendt and K. D. Jordan, Chem. Phys. 89, 245 (1984). 29. H. Sasada, T. Amano, C. Jarman and P. F. Bernath, J. Chem. Phys. 94, 240 1 (199 1). J. Reynolds (Editor) © 1 993 Elsevier Science Publishers B. V. All rights reserved. N. M. Neumark* 3. 1 Introduction Elemental clusters have received a great deal of experimental and theoretical attention in re­ cent years.

8 1 , 4477 (1959); S. J. Strickler and K. S. Pitzer, in Molecular Orbitals in Chemistry, Physics and Biology, B. Pullman and P. 0. LOwdin, eds. (Academic, New York, 1964). 5. D. H. Magers, R. J. Harrison and R. J. Bartlett, J. Chem. Phys. 84, 3284 (1986). 6. W. Weltner Jr. and D. , J. Chem. Phys. 45, 3096 (1966); W. R. M. Graham, K. I. Dismuke and W. , J. Am. Chem. Soc. 93, 4688 (197 1); , Astrophys. J. 204, 301 ( 1976). 7. R. J. Bartlett, Ann. Rev. Phys. Chem. 32, 359 (1981). 8. N. C. Handy, R.

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